A textbook of organic chemistry by Chamberlain JS

By Chamberlain JS

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20. Receptors 61 and 63 (but not 62) were shown to complex more tightly aromatic ammonium in chloroform, using the proposed interactions. Extensive conformational studies by CD and NMR spectroscopy confirmed that the receptor framework existed in a B-sheet conformation in which only 61 24 The Development of Peptide Nanostructure 1010 109 O ,d v t~ 108 107 06r j 105 . nPrNH 2 2 3 ~ ~~i 4 5 6 7 8 =ll H2N-(CH2)n-NH2 Fig. 19. Binding constants observed for the complexation of diamines by the bis-zincporphyrin peptide 58 (striped columns) and a mono-zincporphyrin tripeptide analog (BOC-A-Zn'porphyrinE-A-OMe) (solid columns).

P450 A n a l o g u e s with S u b s t r a t e R e c o g n i t i o n Sites . . . . E l e c t r o n Deficient M e t a l P o r p h y r i n s ............... Reductive O x y g e n Cleavage . . . . . . . . . . . 3 Final Comment . . . . . . . . . . . . . . . . 92 4 References . . . . . . . . . . . . . . . . . 93 Topics in Current Chemistry, Vol. -D. 1 Introduction The significance of cytochrome P450 catalyzed reactions has now been recognized for more than 30 years [1] as one of nature's most common and sophisticated methods to oxidize endogeneous compounds in procaryotic and eucaryotic organisms.

Benson DR, Hart BR, Zhu X, Doughty MB (1995) J Am Chem Soc 117:8502 69. Mihara H, Nishino N, Hasegawa R, Fujimoto T, Usui S, Ishida H, Ohkubo K (1992) Chem Lett 1992:1813 70. (a) Morii H, Ichimura K, Uedaira H (1990) Chem Lett 1990: 1987; (b) ibid (1991) Proteins Struc Funct Gen 11:133 71. Cuenoud B, Schepartz A (1993) Science 259:510 72. Ueno M, Murakami A, Makino K, Morii T (1993) J Am Chem Soc 115:12575 73. Hahn KW, Klis WA, Stewart JM (1990) Science 248:1544 74. (a) Johnsson K, Alleman RK, Widmer H, Benner SA (1993) Nature 365: 530; (b) Johnsson K, Alleman RK, Benner SA (1990) In: Bleasdale C, Golding BT (eds) Molecular Mechanisms in Bioorganic Processes, RSC, Cambridge, UK, p 166 37 Cytochrome P450: Significance, Reaction Mechanisms and Active Site Analogues Wolf-Dietrich Woggon I n s t i t u t F i i r O r g a n i s c h e C h e m i e d e r Universitiit Basel St.

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